Gold nanorods and nanospheroids for enhancing spontaneous emission
Золотые наностержни и наносфероиды для усиления спонтанного излучения
2008-10-28
SCID: 54.1/83r6ttjt
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finite-difference time-domaingold nanorodsgold nanospheroidsradiative decay ratespontaneous emission enhancement
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Abstract (AI)
We compute the radiative decay rate and the quantum efficiency for an emitter coupled to gold nanorods and nanospheroids using the body-of-revolution finite-difference time-domain method. We study these quantities as a function of the nanoparticle aspect ratio and volume, showing that large enhancements can be achieved with realistic parameters. Moreover, we find that nanospheroids exhibit better performances than nanorods for applications in the visible and near-infrared spectral range.
Key Findings
1
Gold nanospheroids outperform nanorods for spontaneous-emission enhancement in the visible and near-infrared spectral ranges.
2
Large spontaneous-emission enhancements are achievable with realistic gold nanoparticle parameters.
3
Radiative enhancement and quantum efficiency depend strongly on nanoparticle aspect ratio and volume.
4
The study computes radiative decay rates and quantum efficiencies for emitters coupled to gold nanorods and nanospheroids using body-of-revolution FDTD.
Research Object
gold nanorods and nanospheroids coupled to an emitter
Research Subject
radiative decay rate and quantum efficiency, including their dependence on nanoparticle aspect ratio and volume and the comparative emission-enhancement performance of nanorods versus nanospheroids
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Publication Date
2008-10-28
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