Implementation of Americium Separation from a PUREX Raffinate

Реализация разделения америция из раффината PUREX
C. Sorel, Marie-Jordane Bollesteros, Jean-Noël Calor, Sylvain Costenoble, Marc Montuir, V. Pacary, Fabien Burdet, Denis Espinoux, Xavier Hérès, Catherine Eysseric
2012-01-01

EXAm processPUREX raffinateamericium separationliquid-liquid extractionminor actinides
Recovering of minor actinides from spent nuclear fuel is investigated for heterogeneous recycling in Generation-IV reactors. After plutonium, americium is the main contributor to residual heat of long term radioactive waste which determines waste density within geological repository. Selective americium separation (EXAm process) by liquid-liquid extraction from a PUREX raffinate was studied. Two experiments were performed in ATALANTE facilities. The first test, on surrogate solution, validated the americium extraction performance. The second trial was carried out in the high-level shielded process line from a genuine PUREX raffinate. Tools used to manage the process are introduced to show performance process achievement.
1
A second trial processed genuine high-level PUREX raffinate in a shielded process line, confirming applicability to real feedstock.
2
Process management tools were introduced and used to demonstrate achievement of the EXAm process performance.
3
Selective americium separation from PUREX raffinate by liquid-liquid extraction (EXAm process) was studied for heterogeneous recycling in Generation-IV reactors.
4
Two experiments in ATALANTE facilities demonstrated the process: a surrogate-solution test validated americium extraction performance.

Selective americium separation from a PUREX raffinate by liquid–liquid extraction (EXAm process)

Performance and implementation of the EXAm liquid–liquid extraction process for recovering americium from PUREX raffinate, validated on surrogate and genuine high-level solutions including process management tools and operational performance in ATALANTE facilities

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2012-01-01
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Authors
C. Sorel
Marie-Jordane Bollesteros
Jean-Noël Calor
Sylvain Costenoble
Marc Montuir
V. Pacary
Fabien Burdet
Denis Espinoux
Xavier Hérès
Catherine Eysseric
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