Spontaneous emission of an atom in the presence of nanobodies

Спонтанное излучение атома в присутствии нанообъектов
В. В. Климов, M. Ducloy, V. S. Letokhov
2001-07-31

nanobodiesnanocylindernanospheroidnonradiative decayspontaneous emission
The effect of nanobodies, i.e., the bodies whose size is small compared to the emission wavelength, on spontaneous emission of an atom located near them is considered. The results of calculations performed within the framework of quantum and classical electrodynamics are presented both in analytic and graphical forms and can be readily used for planning experiments and analysis of experimental data. It is shown that nanobodies can be used to control efficiently the rate of spontaneous transitions. Thus, an excited atom located near a nanocylinder or a nanospheroid pole, whose transition dipole moment is directed normally to the nanobody surface, can decay with the rate that is tens and hundreds times higher than the decay rate in a free space. In the case of some (negative) dielectric constants, the decay rate can increase by a factor of 10 5 —10 6 and more. On the other hand, the decay of an excited atom whose transition dipole moment is directed tangentially to the nanobody surface substantially slows down. The probability of nonradiative decay of the excited state is shown to increase substantially in the presence of na-nobodies possessing losses.
1
A dipole oriented tangentially to the nanobody surface experiences substantial suppression of excited-state decay.
2
For a dipole oriented normally to a nanocylinder or nanospheroid pole, the decay rate can reach tens or hundreds of times the free-space rate.
3
For certain negative dielectric constants, the spontaneous-decay rate can increase by factors of 10^5–10^6 or more.
4
Lossy nanobodies substantially increase the probability of nonradiative decay.
5
Nanobodies can efficiently control an atom’s spontaneous-transition rate when the atom is located nearby.

an atom located near nanobodies, including nanocylinders and nanospheriods

the effect of nanobody geometry, dielectric constants, losses, and transition-dipole orientation on the atom’s spontaneous-emission rate and radiative versus nonradiative decay

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Publication Date
2001-07-31
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Authors
В. В. Климов
M. Ducloy
V. S. Letokhov
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