Double-slit photoelectron interference in strong-field ionization of the neon dimer

Интерференция фотоэлектронов в двух щелях при ионизации димера неона сильным лазерным полем
Maksim Kunitski, Nicolas Eicke, Pia Huber, Jonas Köhler, Stefan Zeller, Jörg Voigtsberger, Nikolai Schlott, Kevin Henrichs, Hendrik Sann, Florian Trinter, Lothar Ph. H. Schmidt, Anton Kalinin, Markus S. Schöffler, Till Jahnke, Manfred Lein, Reinhard Dörner
2018-12-27

double-slit interferencegerade and ungerade interferencemolecular-frame photoelectron momentum distributionneon dimerstrong-field ionization
Wave-particle duality is an inherent peculiarity of the quantum world. The double-slit experiment has been frequently used for understanding different aspects of this fundamental concept. The occurrence of interference rests on the lack of which-way information and on the absence of decoherence mechanisms, which could scramble the wave fronts. Here, we report on the observation of two-center interference in the molecular-frame photoelectron momentum distribution upon ionization of the neon dimer by a strong laser field. Postselection of ions, which are measured in coincidence with electrons, allows choosing the symmetry of the residual ion, leading to observation of both, gerade and ungerade, types of interference.
1
Coincident detection of ions and electrons enables postselection based on the residual ion’s symmetry.
2
Postselection reveals both gerade and ungerade interference patterns in neon-dimer photoelectron emission.
3
The results demonstrate that strong-field ionization of a diatomic molecule can preserve and expose wave interference associated with emission from two centers.
4
Two-center (double-slit) interference was observed in molecular-frame photoelectron momentum distributions from strong-field ionization of the neon dimer.

Neon dimer (Ne2) undergoing strong-field ionization

two-center (double-slit) interference in the molecular-frame photoelectron momentum distribution, including gerade and ungerade symmetry effects selected by the residual-ion state

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2018-12-27
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Authors
Maksim Kunitski
Nicolas Eicke
Pia Huber
Jonas Köhler
Stefan Zeller
Jörg Voigtsberger
Nikolai Schlott
Kevin Henrichs
Hendrik Sann
Florian Trinter
Lothar Ph. H. Schmidt
Anton Kalinin
Markus S. Schöffler
Till Jahnke
Manfred Lein
Reinhard Dörner
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