Theory of high-harmonic generation by low-frequency laser fields
Теория генерации высоких гармоник в низкочастотных лазерных полях
1994-03-01
SCID: 54.1/ncdp7qgp
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atomic dipole matrix elementsharmonic cutoffhigh-harmonic generationlow-frequency laser fieldsponderomotive energy (Up)
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Abstract (AI)
We present a simple, analytic, and fully quantum theory of high-harmonic generation by low-frequency laser fields. The theory recovers the classical interpretation of Kulander et al. in Proceedings of the SILAP III Works hop, edited by B. Piraux (Plenum, New York, 1993) and Corkum [Phys. Rev. Lett. 71, 1994 (1993)] and clearly explains why the single-atom harmonic-generation spectra fall off at an energy approximately equal to the ionization energy plus about three times the oscillation energy of a free electron in the field. The theory is valid for arbitrary atomic potentials and can be generalized to describe laser fields of arbitrary ellipticity and spectrum. We discuss the role of atomic dipole matrix elements, electron rescattering processes, and of depletion of the ground state. We present the exact quantum-mechanical formula for the harmonic cutoff that differs from the phenomenological law ${\mathit{I}}_{\mathit{p}}$+3.17${\mathit{U}}_{\mathit{p}}$, where ${\mathit{I}}_{\mathit{p}}$ is the atomic ionization potential and ${\mathit{U}}_{\mathit{p}}$ is the ponderomotive energy, due to the account for quantum tunneling and diffusion effects.
Key Findings
1
A simple, analytic, fully quantum theory of high-harmonic generation (HHG) by low-frequency laser fields is presented.
2
An exact quantum-mechanical formula for the harmonic cutoff is derived that differs from the phenomenological Ip + 3.17 Up law by including quantum tunneling and diffusion effects.
3
Single-atom harmonic spectra cutoff is explained to occur near the ionization energy plus roughly three times the free-electron oscillation energy in the field.
4
The roles of atomic dipole matrix elements, electron rescattering, and ground-state depletion in HHG are analyzed within the theory.
5
The theory is valid for arbitrary atomic potentials and generalizable to laser fields of arbitrary ellipticity and spectrum.
6
The theory recovers and explains the classical three-step interpretation of Kulander et al. and Corkum for HHG.
Research Object
High-harmonic generation (single-atom response) driven by low-frequency laser fields
Research Subject
Quantum theory and mechanisms determining the harmonic spectra and cutoff (including role of atomic dipole matrix elements, electron rescattering, ground-state depletion, quantum tunneling and diffusion) for low-frequency-driven high-harmonic generation, and derivation of an exact quantum-mechanical cutoff formula vs. the phenomenological Ip+3.17Up law
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1994-03-01
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