Triple-q Order in Na2Co2TeO6 from Proximity to Hidden-SU(2)-Symmetric Point

Yuan Li, Lukas Janssen, Wilhelm G. F. Krüger, Wenjie Chen, Xianghong Jin
2023-10-05

SCID:  54.1/zycvsmde
In extended Heisenberg-Kitaev-Gamma-type spin models, hidden-SU(2)-symmetric points are isolated points in parameter space that can be mapped to pure Heisenberg models via nontrivial duality transformations. Such points generically feature quantum degeneracy between conventional single-$\mathbf{q}$ and exotic multi-$\mathbf{q}$ states. We argue that recent single-crystal inelastic neutron scattering data place the honeycomb magnet ${\mathrm{Na}}_{2}{\mathrm{Co}}_{2}{\mathrm{TeO}}_{6}$ in proximity to such a hidden-SU(2)-symmetric point. The low-temperature order is identified as a triple-$\mathbf{q}$ state arising from the N\'eel antiferromagnet with staggered magnetization in the out-of-plane direction via a 4-sublattice duality transformation. This state naturally explains various distinctive features of the magnetic excitation spectrum, including its surprisingly high symmetry and the dispersive low-energy and flat high-energy bands. Our result demonstrates the importance of bond-dependent exchange interactions in cobaltates, and illustrates the intriguing magnetic behavior resulting from them.
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2023-10-05
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Yuan Li
Lukas Janssen
Wilhelm G. F. Krüger
Wenjie Chen
Xianghong Jin
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