A direct recycling case study from a lithium-ion battery recall

Практическое исследование прямой переработки литий-ионных аккумуляторов, отозванных с рынка
Steve Sloop, Lauren Crandon, Marshall J. Allen, Kara Koetje, L. E. Reed, Linda Gaines, Weekit Sirisaksoontorn, Michael M. Lerner
2020-01-09

cathode healingdirect recyclingelectrode harvestingfroth flotationlithium-ion batteries
Direct recycling of lithium-ion is a promising method for manufacturing sustainability. It is more efficient than classical methods because it recovers the functional cathode particle without decomposition into substituent elements or dissolution and precipitation of the whole particle. This case study of cathode-healing™ applied to a battery recall demonstrates an industrial model for recycling of lithium-ion, be it consumer electronic or electric vehicle (EV) batteries. The comprehensive process includes extraction of electrolyte with carbon dioxide, industrial shredding, electrode harvesting, froth flotation, cathode-healing™ and finally, building new cells with recycled cathode and anode. The final products demonstrated useful capability in the first full cells made from direct recycled cathodes and anodes from an industrial source. The lessons learned on recycling the prototypical chemistry are preliminarily applied to EV relevant chemistries.
1
Direct recycling can improve manufacturing sustainability by preserving functional lithium-ion cathode particles rather than decomposing and reconstituting their constituent elements.
2
Lessons from recycling the prototype battery chemistry were preliminarily extended to chemistries relevant to electric-vehicle batteries.
3
New full cells assembled with directly recycled cathodes and anodes from an industrial battery recall demonstrated useful electrochemical capability.
4
The case study demonstrates an industrial recycling workflow combining carbon-dioxide electrolyte extraction, shredding, electrode harvesting, froth flotation, cathode healing, and cell rebuilding.

Direct recycling of recalled lithium-ion batteries, including their cathode and anode materials

Industrial direct-recycling process performance, including cathode healing and the fabrication and electrochemical capability of new cells using recovered electrode materials

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Publication Date
2020-01-09
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Authors
Steve Sloop
Lauren Crandon
Marshall J. Allen
Kara Koetje
L. E. Reed
Linda Gaines
Weekit Sirisaksoontorn
Michael M. Lerner
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